Mercury Sorbent Tube Method (40CFR75, Appendix K)
The
Appendix K Sorbent Tube Method was developed with the critical support of ERPI, and is designed
for the sampling of mercury emissions in combustion flue gas streams using dry
sorbent traps, followed by analysis of each trap by EPA Method 1631, Revision E,
using Cold Vapor Atomic Fluorescence Spectrometry (CVAFS). Known volumes of flue
gas are extracted from a duct through a specially designed, low mercury blank,
sorbent trap with a nominal flow rate of 0.2 to 0.6 L/min. The analyte measured
by this method is total vapor-phase mercury, which represents the sum of
elemental and oxidized forms of mercury. Mercury concentrations are determined
on a mass basis (ug/m3) and then combined with flue gas flow data (m3/min) to
calculate the continuous mass emission rate of total vapor phase mercury.
Fluegas Absorbent Mercury Speciation (FAMS) Method
The FAMS method relies on sequential selective capture to separate and
quantify three mercury species, particulate Hg (Hgp), gaseous oxidized (Hg2+),
and gaseous elemental (Hg0). A known, precise volume (±0.1 liter) of gas is
pulled through the FAMS sorbent train using standard sampling equipment
including a quartz probe liner, heated probe, silica-gel water trap, mass flow
meter and pump. The temperature of the FAMS sorbent train is kept at 95 ± 5 °C
during sampling to avoid water condensation in the trap. The sorbed Hg0 on the
chemically impregnated carbon and the PHg on the glass wool plug is leached of
collected Hg in the clean lab using hot-refluxing HNO3/H2SO4, then further
oxidation in BrCl solution. The sorbed Hg(II) on the KCl trap is dissolved in
(v/v) BrCl solution. Aliquots of all three Hg species digests are analyzed using
EPA Method 1631.